The System

The sources of data used to determine mixture parameters W, Q and U in the activity coefficient equations for this ternary (3 ion) system are listed in Table 5 of Clegg et al. (1997). Fits of the model are described in that paper, and in section 3.17 of Clegg et al. (1998b). The following types of data were considered:

1. Saturation with respect to the solids Na2SO4.10H2O(s), Na2SO4(s), and NaCl(s) in the ternary solution.
2. Osmotic coefficients from isopiestic experiments.
3. Mean activity coefficients of NaCl from electromotive force measurements.
4. Osmotic coefficients from electrodynamic balance measurements (not fitted).

References:
S. L. Clegg, P. Brimblecombe, Z. Liang and C. K. Chan (1997) Aerosol Science and Technology 27, 345-366.
S. L. Clegg, P. Brimblecombe and A. S. Wexler (1998b) J. Phys. Chem. A 102, 2155-2171.

Weights

The values listed in the tables below are based upon those used in the fits of the model. However, they have been normalised for each type of measurement so that the maximum weight for a data point in each table is always unity. Points given zero weight are those which either appear to be in error, or are used for comparison only (and were not fitted). Points with a weight of "-" are outside the temperature or concentration limits of the current model, and have not been assessed for accuracy.

The Data

The experimental data used to fit the activity coefficient model are listed in the tables below. Notes at the end of each one define the tabulated quantities, and identify the sources of the measurements. Electrodynamic balance measurements (yielding osmotic coefficients of supersaturated solutions) used by Clegg et al. (1997) are given in Table 6.

(1) Solubilities of Solid Phases

    mNaCl     mNa2SO4     t     solid   ref.      weight   
    0.505433  1.87248   25.0      10   a(3244)      1.0     
    0.990716  1.71198   25.0      10   a(3244)      1.0     
    3.271082  1.45905   25.0      10   a(3244)      1.0     
    3.271082  1.45905   25.0       1   a(3244)      1.0     
    3.971774  1.14604   25.0       1   a(3244)      1.0     
    5.314481  0.70303   25.0       1   a(3244)      1.0     
    5.543115  0.69942   25.0       1   a(3244)      1.0     
    5.646010  0.69286   25.0       2   a(3244)      1.0     
    5.646010  0.69286   25.0       1   a(3244)      1.0     
    5.782363  0.46869   25.0       2   a(3244)      1.0     
    5.918694  0.23798   25.0       2   a(3244)      1.0     
    6.093704  0.00000   25.0       2   a(3244)      0.0     
    6.172644  0.00000   25.0       2   a(3249)      0.0     
    5.844711  0.32232   25.0       2   a(3249)      1.0     
    5.732748  0.50719   25.0       2   a(3249)      1.0     
    5.655787  0.68884   25.0       2   a(3249)      1.0     
    5.655787  0.68884   25.0       1   a(3249)      1.0     
    3.664344  1.41005   25.0       1   a(3249)      1.0     
    3.491661  1.49944   25.0      10   a(3249)      1.0     
    3.491661  1.49944   25.0       1   a(3249)      1.0     
    3.056661  1.53490   25.0      10   a(3249)      1.0     
    0.000000  1.97070   25.0      10   a(3249)      0.0     
    6.166309  0.00000   25.0       2   a(3252)      0.0     
    5.804655  0.29160   25.0       2   a(3252)      1.0     
    5.599883  0.68177   25.0       2   a(3252)      1.0     
    5.599883  0.68177   25.0       1   a(3252)      1.0     
    4.938302  0.85361   25.0       1   a(3252)      1.0     
    4.571608  1.00448   25.0       1   a(3252)      1.0     
    3.132563  1.53950   25.0       1   a(3252)      1.0     
    3.270445  1.50079   25.0       1   a(3252)      1.0     
    3.270445  1.50079   25.0      10   a(3252)      1.0     
    2.233838  1.47675   25.0      10   a(3252)      1.0     
    0.929065  1.65701   25.0      10   a(3252)      1.0     
    0.000000  1.93280   25.0      10   a(3252)      0.0     
    5.421486  0.68710   25.0       2   a(3253)      1.0     
    5.421486  0.68710   25.0       1   a(3253)      1.0     
    4.374024  1.04813   25.0       1   a(3253)      1.0     
    3.383643  1.51147   25.0       1   a(3253)      1.0     
    3.383643  1.51147   25.0      10   a(3253)      1.0     
    1.392279  1.62610   25.0      10   a(3253)      1.0     
    0.464267  1.86467   25.0      10   a(3253)      1.0     
    0.000000  1.97416   25.0      10   a(3253)      0.0     
    1.716984  1.47556   25.0      10   a(3258)      1.0     
    3.494615  1.43780   25.0      10   a(3258)      1.0     
    3.405431  1.48148   25.0      10   a(3258)      1.0     
    3.270445  1.50079   25.0      10   a(3258)      1.0     
    3.494615  1.43780   25.0       1   a(3258)      1.0     
    3.405431  1.48148   25.0       1   a(3258)      1.0     
    3.270445  1.50079   25.0      10   a(3258)      1.0     
    4.422090  1.02835   25.0       1   a(3258)      1.0     
    5.530076  0.70764   25.0       1   a(3258)      1.0     
    5.541607  0.69291   25.0       1   a(3258)      1.0     
    5.599883  0.68177   25.0       1   a(3258)      1.0     
    5.530076  0.70764   25.0       2   a(3258)      1.0     
    5.541607  0.69291   25.0       2   a(3258)      1.0     
    5.599883  0.68177   25.0       2   a(3258)      1.0     
    5.842395  0.32734   25.0       2   a(3258)      1.0     
    6.207548  0.00000   25.0       2   a(3272)      0.0     
    6.084059  0.25375   25.0       2   a(3272)      1.0     
    5.579487  0.69730   25.0       2   a(3272)      1.0     
    5.579487  0.69730   25.0       1   a(3272)      1.0     
    4.814911  0.99902   25.0       1   a(3272)      0.0     
    3.493591  1.49723   25.0      10   a(3272)      1.0     
    3.493591  1.49723   25.0       1   a(3272)      1.0     
    3.585649  1.42555   25.0      10   a(3272)      1.0     
    2.022692  1.55225   25.0      10   a(3272)      1.0     
    0.855799  1.70593   25.0      10   a(3272)      1.0     
    0.000000  1.96609   25.0      10   a(3272)      0.0     
    0.000000  1.97070   25.0      10   a(3282)      0.0     
    1.132234  1.73673   25.0      10   a(3282)      1.0     
    1.402958  1.69257   25.0      10   a(3282)      1.0     
    1.590133  1.66507   25.0      10   a(3282)      1.0     
    2.092133  1.61026   25.0      10   a(3282)      1.0     
    2.335724  1.57994   25.0      10   a(3282)      1.0     
    3.055807  1.53250   25.0      10   a(3282)      1.0     
    3.390392  1.51431   25.0      10   a(3282)      1.0     
    3.390392  1.51431   25.0       1   a(3282)      1.0     
    3.776562  1.33438   25.0       1   a(3282)      1.0     
    4.634081  0.98858   25.0       1   a(3282)      1.0     
    5.713694  0.72862   25.0       1   a(3282)      0.0     
    5.713694  0.72862   25.0       2   a(3282)      1.0     
    5.703049  0.56422   25.0       2   a(3282)      1.0     
    5.758147  0.44544   25.0       2   a(3282)      1.0     
    5.933289  0.38581   25.0       2   a(3282)      1.0     
    6.163143  0.00000   25.0       2   a(3282)      0.0     
    0.0000    0.6431    10.00     10   a(3242)       -      
    0.7250    0.3700    10.00     10   a(3242)       -      
    1.6416    0.3349    10.00     10   a(3242)       -      
    2.6778    0.2813    10.00     10   a(3242)       -      
    3.7321    0.2798    10.00     10   a(3242)       -      
    4.8118    0.2924    10.00     10   a(3242)       -      
    5.1507    0.3057    10.00     10   a(3242)       -      
    5.5217    0.3228    10.00     10   a(3242)       -      
    5.7754    0.3345    10.00     10   a(3242)       -      
    0.0000    1.5017    21.50     10   a(3242)       -      
    1.5491    1.0898    21.50     10   a(3242)       -      
    2.9902    0.9662    21.50     10   a(3242)       -      
    3.4900    0.9586    21.50     10   a(3242)       -      
    4.4502    1.0585    21.50      1   a(3242)       -      
    4.5363    1.0161    21.50      1   a(3242)       -      
    4.7449    0.9429    21.50      1   a(3242)       -      
    5.3444    0.7470    21.50      1   a(3242)       -      
    5.4410    0.7242    21.50      1   a(3242)       -      
    5.4912    0.5926    21.50      2   a(3242)       -      
    5.7651    0.3333    21.50      2   a(3242)       -      
    5.8300    0.1946    21.50      2   a(3242)       -      
    6.0714    0.0000    21.50      2   a(3242)       -      
    0.0000    2.1881    27.00     10   a(3242)       -      
    0.4541    2.0218    27.00     10   a(3242)       -      
    0.9043    1.9126    27.00     10   a(3242)       -      
    1.3518    1.8308    27.00     10   a(3242)       -      
    2.7589    1.7475    27.00     10   a(3242)       -      
    3.2330    1.5051    27.00      1   a(3242)       -      
    3.3590    1.4146    27.00      1   a(3242)       -      
    3.5539    1.3578    27.00      1   a(3242)       -      
    5.5320    0.6712    27.00      1   a(3242)       -      
    0.0000    2.7939    30.00     10   a(3242)       -      
    0.4189    2.6922    30.00     10   a(3242)       -      
    0.9605    2.5693    30.00     10   a(3242)       -      
    1.3539    2.5312    30.00     10   a(3242)       -      
    1.8157    2.2273    30.00      1   a(3242)       -      
    2.1148    2.1028    30.00      1   a(3242)       -      
    2.6761    1.7606    30.00      1   a(3242)       -      
    3.1534    1.4992    30.00      1   a(3242)       -      
    3.5331    1.3416    30.00      1   a(3242)       -      
    5.4847    0.6357    30.00      1   a(3242)       -      
    0.0000    3.4053    33.00      1   a(3242)       -      
    0.2175    3.2742    33.00      1   a(3242)       -      
    0.3398    3.1779    33.00      1   a(3242)       -      
    0.4519    3.1029    33.00      1   a(3242)       -      
    0.5949    2.9988    33.00      1   a(3242)       -      
    2.0765    2.0633    33.00      1   a(3242)       -      
    3.7396    1.1843    33.00      1   a(3242)       -      
    5.6188    0.6171    33.00      1   a(3242)       -      
    5.8158    0.3260    33.00      2   a(3242)       -      
    5.9483    0.1936    33.00      2   a(3242)       -      
    0.0000    3.3698    35.00      1   a(3242)       -      
    0.3616    2.9336    35.00      1   a(3242)       -      
    2.3203    1.8475    35.00      1   a(3242)       -      
    3.2112    1.3896    35.00      1   a(3242)       -      
    5.4597    0.5833    35.00      1   a(3242)       -      
    6.0934    0.0000    35.00      2   a(3242)       -      
     5.616    0.566     14.80      2   a(3243)       -      
     5.626    0.567     17.90      2   a(3243)       -      
     5.663    0.566     24.85      2   a(3243)       -      
     5.673    0.567     25.60      2   a(3243)       -      
     5.686    0.567     27.75      2   a(3243)       -      
     5.696    0.567     32.18      2   a(3243)       -      
     5.737    0.567     34.28      2   a(3243)       -      
     1.0694   0.6381    15.00     10   a(3246)       -      
     2.3837   0.5002    15.00     10   a(3246)       -      
     3.4677   0.4673    15.00     10   a(3246)       -      
     4.8818   0.5024    15.00     10   a(3246)       -      
     5.6393   0.5595    15.00     10   a(3246)       -      
     5.6393   0.5595    15.00      2   a(3246)       -      
     5.9473   0.2194    15.00      2   a(3246)       -      
     6.1060   0.0000    15.00      2   a(3247)       -      
     5.9473   0.2194    15.00      2   a(3247)       -      
     5.6393   0.5595    15.00      2   a(3247)       -      
     5.6393   0.5595    15.00     10   a(3247)       -      
     4.8818   0.5024    15.00     10   a(3247)       -      
     3.4677   0.4673    15.00     10   a(3247)       -      
     2.3837   0.5002    15.00     10   a(3247)       -      
     1.0694   0.6381    15.00     10   a(3247)       -      
     0.0000   0.9149    15.00     10   a(3247)       -      
     5.562    0.686     25.00      2   a(3247)       -      
     5.562    0.686     25.00      1   a(3247)       -      
     3.321    1.509     25.00      1   a(3247)       -      
     3.321    1.509     25.00     10   a(3247)       -      
     5.695    0.614     35.00      1   a(3247)       -      
     5.695    0.614     35.00      2   a(3247)       -      
     6.106    0.000      0.00      2   a(3249)       -      
     6.005    0.114      0.00      2   a(3249)       -      
     6.005    0.114      0.00     10   a(3249)       -      
     0.000    0.350      0.00     10   a(3249)       -      
     6.0005   0.1350     0.00      2   a(3253)       -      
     6.0005   0.1350     0.00     10   a(3253)       -      
     2.0852   0.1203     0.00     10   a(3253)       -      
     5.744    0.611     40.00      1   a(3253)       -      
     5.744    0.611     40.00      2   a(3253)       -      
     5.996    0.522     60.00      1   a(3253)       -      
     5.996    0.522     60.00      2   a(3253)       -      
     6.211    0.505     80.00      1   a(3253)       -      
     6.211    0.505     80.00      2   a(3253)       -      
     4.2297   0.0986     0.00     10   a(3254)       -      
     2.8727   0.1016     0.00     10   a(3254)       -      
     6.641    0.000     94.50      2   a(3254)       -      
     6.597    0.243     94.50      2   a(3254)       -      
     6.326    0.446     94.50      2   a(3254)       -      
     6.326    0.446     94.50      1   a(3254)       -      
     3.917    0.942     94.50      1   a(3254)       -      
     3.615    1.033     94.50      1   a(3254)       -      
     0.556    2.594     94.50      1   a(3254)       -      
     0.000    3.053     94.50      1   a(3254)       -      
     6.169    0.000     35.00      2   a(3256)       -      
     5.615    0.607     35.00      2   a(3256)       -      
     5.615    0.607     35.00      1   a(3256)       -      
     0.000    3.483     35.00      1   a(3256)       -      
     5.061    0.011    -21.70      0   a(3258)       -      
     5.061    0.011    -21.70      3   a(3258)       -      
     5.061    0.011    -21.70     10   a(3258)       -      
     5.257    0.029    -21.32      0   a(3258)       -      
     5.257    0.029    -21.32      3   a(3258)       -      
     5.257    0.029    -21.32     10   a(3258)       -      
     5.082    0.000    -21.60      0   a(3258)       -      
     5.082    0.000    -21.60      3   a(3258)       -      
     5.163    0.000    -20.94      0   a(3258)       -      
     5.163    0.000    -20.94      3   a(3258)       -      
     0.000    0.277     -1.20      0   a(3258)       -      
     0.000    0.277     -1.20     10   a(3258)       -      
     5.905    0.133     -0.10      3   a(3258)       -      
     5.905    0.133     -0.10     10   a(3258)       -      
     5.905    0.133     -0.10      2   a(3258)       -      
     6.054    0.127      0.00      3   a(3258)       -      
     6.054    0.127      0.00     10   a(3258)       -      
     6.054    0.127      0.00      2   a(3258)       -      
     1.723    0.325     10.20     10   a(3258)       -      
     3.700    0.289     10.20     10   a(3258)       -      
     5.750    0.330     10.20     10   a(3258)       -      
     5.750    0.330     10.20      2   a(3258)       -      
     5.561    0.534     15.00     10   a(3258)       -      
     5.561    0.534     15.00      2   a(3258)       -      
     1.667    0.719     17.50     10   a(3258)       -      
     3.790    0.627     17.50     10   a(3258)       -      
     5.421    0.731     17.50     10   a(3258)       -      
     5.421    0.731     17.50      2   a(3258)       -      
     5.441    0.760     17.90     10   a(3258)       -      
     5.441    0.760     17.90      1   a(3258)       -      
     5.441    0.760     17.90      2   a(3258)       -      
     0.811    2.591     30.00     10   a(3258)       -      
     1.402    2.539     30.00     10   a(3258)       -      
     1.402    2.539     30.00      1   a(3258)       -      
     2.916    1.593     30.00      1   a(3258)       -      
     4.260    0.945     30.00      1   a(3258)       -      
     5.596    0.669     30.00      1   a(3258)       -      
     5.596    0.669     50.00      2   a(3258)       -      
     1.883    2.052     50.00      1   a(3258)       -      
     3.795    1.096     50.00      1   a(3258)       -      
     5.861    0.554     50.00      1   a(3258)       -      
     5.861    0.554     50.00      2   a(3258)       -      
     6.033    0.250     50.00      2   a(3258)       -      
     1.830    1.912     75.00      1   a(3258)       -      
     3.852    0.980     75.00      1   a(3258)       -      
     6.206    0.500     75.00      1   a(3258)       -      
     6.206    0.500     75.00      2   a(3258)       -      
     6.321    0.211     75.00      2   a(3258)       -      
     7.861    3.667     94.50      1   a(3258)       -      
     3.615    1.033     94.50      1   a(3258)       -      
     6.326    0.446     94.50      1   a(3258)       -      
     6.326    0.446     94.50      2   a(3258)       -      
     6.597    0.243     94.50      2   a(3258)       -      
     1.780    1.776    100.00      1   a(3258)       -      
     4.322    0.846    100.00      1   a(3258)       -      
     6.368    0.456    100.00      1   a(3258)       -      
     6.368    0.456    100.00      2   a(3258)       -      
     6.559    0.183    100.00      2   a(3258)       -      
     6.586    0.514    109.10      1   a(3258)       -      
     6.586    0.514    109.10      2   a(3258)       -      
     5.6852   0.0528    -8.00      3   a(3259)       -      
     5.6852   0.0528    -8.00     10   a(3259)       -      
     3.4602   0.0511    -8.00     10   a(3259)       -      
     2.2003   0.0520    -8.00     10   a(3259)       -      
     2.2003   0.0520    -8.00      0   a(3259)       -      
     5.7766   0.0673    -5.00      3   a(3259)       -      
     5.7766   0.0673    -5.00     10   a(3259)       -      
     3.5487   0.0634    -5.00     10   a(3259)       -      
     2.4362   0.0608    -5.00     10   a(3259)       -      
     1.4217   0.0716    -5.00     10   a(3259)       -      
     1.3379   0.0759    -5.00     10   a(3259)       -      
     1.3379   0.0759    -5.00      0   a(3259)       -      
     0.887    0.101     -3.50     10   a(3259)       -      
     0.887    0.101     -3.50      0   a(3259)       -      
     6.0603   0.1876     5.00      2   a(3259)       -      
     6.0603   0.1876     5.00     10   a(3259)       -      
     5.3803   0.1783     5.00     10   a(3259)       -      
     3.2121   0.1594     5.00     10   a(3259)       -      
     2.6675   0.1644     5.00     10   a(3259)       -      
     0.7762   0.2630     5.00     10   a(3259)       -      
     0.0000   0.5129     5.00     10   a(3259)       -      
     5.580    0.543     15.00      2   a(3259)       -      
     5.580    0.543     15.00     10   a(3259)       -      
     1.284    2.595     30.00      1   a(3259)       -      
     1.284    2.595     30.00     10   a(3259)       -      
     2.098    2.066     30.00      1   a(3259)       -      
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     0.000    0.3181     0.00     10   a(3284)       -      
     6.106    0.0000     5.00      2   a(3284)       -      
     5.751    0.1638     5.00      2   a(3284)       -      
     5.751    0.1638     5.00     10   a(3284)       -      
     5.482    0.1521     5.00     10   a(3284)       -      
     3.317    0.1554     5.00     10   a(3284)       -      
     2.569    0.1543     5.00     10   a(3284)       -      
     1.230    0.1943     5.00     10   a(3284)       -      
     0.000    0.4635     5.00     10   a(3284)       -      
     6.099    0.0000    10.00      2   a(3284)       -      
     5.770    0.3342    10.00      2   a(3284)       -      
     5.770    0.3342    10.00     10   a(3284)       -      
     5.514    0.3231    10.00     10   a(3284)       -      
     5.146    0.3053    10.00     10   a(3284)       -      
     4.808    0.2920    10.00     10   a(3284)       -      
     3.729    0.2792    10.00     10   a(3284)       -      
     2.674    0.2809    10.00     10   a(3284)       -      
     1.641    0.3347    10.00     10   a(3284)       -      
     0.732    0.4518    10.00     10   a(3284)       -      
     0.000    0.6428    10.00     10   a(3284)       -      
     5.873    0.000     -5.00      3   a(3284)       -      
     5.433    0.067     -5.00      3   a(3284)       -      
     4.939    0.0488    -5.00      3   a(3284)       -      
     4.939    0.0488    -5.00     10   a(3284)       -      
     3.133    0.0450    -5.00     10   a(3284)       -      
     1.588    0.0472    -2.30      0   a(3284)       -      
     1.588    0.0472    -2.30     10   a(3284)       -      
     0.000    0.2948    -1.10      0   a(3284)       -      
     0.000    0.2948    -1.10     10   a(3284)       -      
     3.489    1.440     24.75      1   a(3245)       -      
     3.489    1.440     24.75     10   a(3245)       -      
     2.763    1.782     26.75      1   a(3245)       -      
     2.763    1.782     26.75     10   a(3245)       -      
     1.831    2.301     28.95      1   a(3245)       -      
     1.831    2.301     28.95     10   a(3245)       -      
     1.791    2.323     29.05      1   a(3245)       -      
     1.791    2.323     29.05     10   a(3245)       -      
     0.000    3.491     32.45      1   a(3245)       -      
     0.000    3.491     32.45     10   a(3245)       -      
     5.980    0.000      0.00      2   a(3248)       -      
     5.900    0.120      0.00      2   a(3248)       -      
     5.900    0.120      0.00     10   a(3248)       -      
     0.000    0.325      0.00     10   a(3248)       -      
     6.097    0.000     25.00      2   a(3248)       -      
     5.503    0.691     25.00      2   a(3248)       -      
     5.503    0.691     25.00      1   a(3248)       -      
     3.220    1.526     25.00      1   a(3248)       -      
     3.220    1.526     25.00     10   a(3248)       -      
     0.000    1.966     25.00     10   a(3248)       -      
     6.245    0.000     50.00      2   a(3248)       -      
     5.766    0.517     50.00      2   a(3248)       -      
     5.766    0.517     50.00      1   a(3248)       -      
     0.000    3.157     50.00      1   a(3248)       -      
     6.459    0.000     75.00      2   a(3248)       -      
     6.067    0.470     75.00      2   a(3248)       -      
     6.067    0.470     75.00      1   a(3248)       -      
     0.000    3.056     75.00      1   a(3248)       -      
     6.742    0.000    100.00      2   a(3248)       -      
     6.256    0.451    100.00      2   a(3248)       -      
     6.256    0.451    100.00      1   a(3248)       -      
     0.000    2.934    100.00      1   a(3248)       -      
     6.1598   0.0000    20.00      2   a(3261)       -      
     5.4412   0.7744    20.00      2   a(3261)       -      
     5.4412   0.7744    20.00      1   a(3261)       -      
     4.9621   0.9153    20.00      1   a(3261)       -      
     4.9621   0.9153    20.00     10   a(3261)       -      
     4.4830   0.8519    20.00     10   a(3261)       -      
     3.4906   0.8237    20.00     10   a(3261)       -      
     2.0191   0.8801    20.00     10   a(3261)       -      
     0.0000   1.3729    20.00     10   a(3261)       -      
     6.211    0.000     35.00      2   a(3261)       -      
     5.749    0.648     35.00      2   a(3261)       -      
     5.749    0.648     35.00      1   a(3261)       -      
     0.000    3.569     35.00      1   a(3261)       -      
     6.245    0.000     50.00      2   a(3261)       -      
     5.766    0.514     50.00      2   a(3261)       -      
     5.766    0.514     50.00      1   a(3261)       -      
     0.000    3.281     50.00      1   a(3261)       -      
     6.468    0.000     75.00      2   a(3261)       -      
     6.074    0.479     75.00      2   a(3261)       -      
     6.074    0.479     75.00      1   a(3261)       -      
     0.000    3.091     75.00      1   a(3261)       -      
     6.382    0.458    100.00      2   a(3261)       -      
     6.382    0.458    100.00      1   a(3261)       -      
     5.5100   0.7880    17.98     10   a(3257)       -      
     5.5100   0.7880    17.98      1   a(3257)       -      
     5.3800   0.8160    18.41     10   a(3257)       -      
     5.3800   0.8160    18.41      1   a(3257)       -      
     4.7200   1.0000    21.00     10   a(3257)       -      
     4.7200   1.0000    21.00      1   a(3257)       -      
     4.4600   1.1100    21.68     10   a(3257)       -      
     4.4600   1.1100    21.68      1   a(3257)       -      
     4.2400   1.2300    22.56     10   a(3257)       -      
     4.2400   1.2300    22.56      1   a(3257)       -      
     3.9300   1.3100    23.48     10   a(3257)       -      
     3.9300   1.3100    23.48      1   a(3257)       -      
     3.7900   1.3300    23.96     10   a(3257)       -      
     3.7900   1.3300    23.96      1   a(3257)       -      
     3.4200   1.4700    25.00     10   a(3257)       -      
     3.4200   1.4700    25.00      1   a(3257)       -      
     3.3000   1.5600    25.50     10   a(3257)       -      
     3.3000   1.5600    25.50      1   a(3257)       -      
     3.0900   1.6300    25.90     10   a(3257)       -      
     3.0900   1.6300    25.90      1   a(3257)       -      
     2.5500   1.9400    27.38     10   a(3257)       -      
     2.5500   1.9400    27.38      1   a(3257)       -      
     1.8000   2.3800    29.02     10   a(3257)       -      
     1.8000   2.3800    29.02      1   a(3257)       -      
     1.4100   2.5700    30.00     10   a(3257)       -      
     1.4100   2.5700    30.00      1   a(3257)       -      
     0.0000   3.5600    32.38     10   a(3257)       -      
     0.0000   3.5600    32.38      1   a(3257)       -      
     0.000    2.974    100.00      1      b          -      
     1.780    1.776    100.00      1      b          -      
     4.322    0.846    100.00      1      b          -      
     6.369    0.457    100.00      1      b          -      
     6.369    0.457    100.00      2      b          -      
     6.368    0.456    100.00      1      b          -      
     6.368    0.456    100.00      2      b          -      
     6.559    0.183    100.00      2      b          -      
     0.000    3.061     75.00      1      b          -      
     1.830    1.912     75.00      1      b          -      
     3.852    0.980     75.00      1      b          -      
     6.206    0.500     75.00      1      b          -      
     6.206    0.500     75.00      2      b          -      
     6.173    0.499     75.00      1      b          -      
     6.173    0.499     75.00      2      b          -      
     6.321    0.211     75.00      2      b          -      
     0.000    3.178     60.00      1      b          -      
     0.000    3.283     50.00      1      b          -      
     1.883    2.052     50.00      1      b          -      
     3.795    1.096     50.00      1      b          -      
     5.862    0.557     50.00      1      b          -      
     5.862    0.557     50.00      2      b          -      
     5.860    0.553     50.00      1      b          -      
     5.860    0.553     50.00      2      b          -      
     6.033    0.250     50.00      2      b          -      
     0.000    3.452     35.00      1      b          -      
     0.000    3.499     32.40      1      b          -      
     0.000    3.499     32.40     10      b          -      
     0.000    2.876     30.00     10      b          -      
     0.811    2.591     30.00     10      b          -      
     1.399    2.539     30.00      1      b          -      
     1.399    2.539     30.00     10      b          -      
     1.407    2.540     30.00      1      b          -      
     1.407    2.540     30.00     10      b          -      
     2.916    1.593     30.00      1      b          -      
     4.260    0.945     30.00      1      b          -      
     5.596    0.669     30.00      1      b          -      
     5.596    0.669     30.00      2      b          -      
     5.564    0.668     30.00      1      b          -      
     5.564    0.668     30.00      2      b          -      
     0.000    1.951     25.00     10      b          -      
     1.717    1.476     25.00      1      b          -      
     1.717    1.476     25.00     10      b          -      
     3.494    1.438     25.00      1      b          -      
     3.494    1.438     25.00     10      b          -      
     3.494    1.438     25.00      1      b          -      
     4.422    1.028     25.00      1      b          -      
     4.422    1.028     25.00      2      b          -      
     5.532    0.711     25.00      1      b          -      
     5.532    0.711     25.00      2      b          -      
     5.495    0.703     25.00      2      b          -      
     0.000    1.361     20.00     10      b          -      
     1.661    0.915     20.00     10      b          -      
     3.023    0.795     20.00     10      b          -      
     4.955    0.916     20.00      1      b          -      
     4.955    0.916     20.00     10      b          -      
     4.955    0.916     20.00      1      b          -      
     4.955    0.916     20.00     10      b          -      
     5.489    0.739     20.00      1      b          -      
     5.489    0.739     20.00      2      b          -      
     5.490    0.740     20.00      1      b          -      
     5.490    0.740     20.00      2      b          -      
     5.833    0.356     20.00      2      b          -      
     5.441    0.760     17.90      1      b          -      
     5.441    0.760     17.90     10      b          -      
     5.441    0.760     17.50      2      b          -      
     0.000    1.127     17.50     10      b          -      
     1.667    0.719     17.50     10      b          -      
     3.790    0.627     17.50     10      b          -      
     5.421    0.731     17.50     10      b          -      
     5.421    0.731     17.50      2      b          -      
     0.000    0.957     15.00     10      b          -      
     5.561    0.535     15.00     10      b          -      
     5.561    0.535     15.00      2      b          -      
     5.560    0.532     15.00     10      b          -      
     5.560    0.532     15.00      2      b          -      
     0.000    0.647     10.20     10      b          -      
     1.724    0.329     10.20     10      b          -      
     3.700    0.289     10.20     10      b          -      
     5.751    0.331     10.20     10      b          -      
     5.751    0.331     10.20      2      b          -      
     5.749    0.329     10.20     10      b          -      
     5.749    0.329     10.20      2      b          -      
     0.000    0.485      6.50     10      b          -      
     5.835    0.239      6.50     10      b          -      
     5.835    0.239      6.50      2      b          -      
     5.907    0.135      0.10      2      b          -      
     5.907    0.135      0.10      5      b          -      
     5.907    0.135      0.10     10      b          -      
     0.000    0.318      0.00     10      b          -      
     3.012    0.093      0.00     10      b          -      
     5.905    0.133      0.00     10      b          -      
     5.905    0.133      0.00      5      b          -      
     0.000    0.277     -1.20     10      b          -      
     0.000    0.277     -1.20      0      b          -      
     5.520    0.074    -10.60     10      b          -      
     5.520    0.074    -10.60      5      b          -      
     2.730    0.158    -10.60      0      b          -      
     2.730    0.158    -10.60     10      b          -      
     5.061    0.011    -21.70      5      b          -      
     5.061    0.011    -21.70     10      b          -      
     5.061    0.011    -21.70      0      b          -      

Notes and References

• Prefix m denotes molality; t - experimental temperature (^oC); solid - identity of the solid which the solution is saturated with respect to; ref. - source of data; weight - the weight given to the data point in the fit of the model (normalised).
• Solids: 0 = ice, 1 = Na2SO4(s), 10 = Na2SO4.10H2O(s), 2 = NaCl(s); 3 = NaCl.2H2O(s).
• Sources: a - H. L. Silcock, Solubilities of Inorganic and Organic Compounds, Vol. 3, Pergamon, Oxford, 1979, (the table numbers are given in parentheses); b - A. Chretien (1929) Ann. Chim. [10] 12, 9-155.
• Data at 25 ^oC that have a weight of '-' were inadvertently excluded from the fit of the model. (However, the amount of data remains substantial at this temperature, as the system has been extensively studied. See Figure 6e of Clegg et al. (1997)).

(2) Osmotic Coefficients from Isopiestic Measurements

     mNaCl    mNa2SO4     osm       t       ref.   weight
    4.14964   0.46161    1.1183     25.0     c      1.0        
    2.04749   0.22776    0.9540     25.0     c      1.0        
    1.34841   0.15000    0.9168     25.0     c      1.0        
    1.01579   0.11300    0.9037     25.0     c      1.0        
    0.80955   0.09005    0.8978     25.0     c      1.0        
    3.56936   0.99619    1.0693     25.0     c      1.0        
    1.77078   0.49421    0.9073     25.0     c      1.0        
    1.16214   0.32435    0.8749     25.0     c      1.0        
    0.87214   0.24341    0.8657     25.0     c      1.0        
    0.69291   0.19339    0.8627     25.0     c      1.0        
    2.02554   2.46854    0.9452     25.0     c      1.0        
    1.02867   1.25364    0.7835     25.0     c      1.0        
    0.66884   0.81512    0.7626     25.0     c      1.0        
    0.49616   0.60468    0.7634     25.0     c      1.0        
    0.39020   0.47554    0.7685     25.0     c      1.0        
    4.64703   0.0        1.1652     25.0     c      0.0        
    2.28440   0.0        0.9977     25.0     c      0.0        
    1.50961   0.0        0.9555     25.0     c      0.0        
    1.14018   0.0        0.9395     25.0     c      0.0        
    0.91120   0.0        0.9307     25.0     c      0.0        
    0.0       4.44527    0.8121     25.0     c      0.0        
    0.0       2.37683    0.6393     25.0     c      0.0        
    0.0       1.53325    0.6272     25.0     c      0.0        
    0.0       1.11557    0.6401     25.0     c      0.0        
    0.0       0.86144    0.6563     25.0     c      0.0             
    1.212     0.0        0.9462     25.0     d      0.0        
    0.966     0.231      0.8737     25.0     d      0.375      
    0.699     0.488      0.8014     25.0     d      0.375      
    0.478     0.720      0.7361     25.0     d      0.375      
    0.237     0.953      0.6891     25.0     d      0.375      
    0.0       1.205      0.6353     25.0     d      0.0        
    1.520     0.0        0.9610     25.0     d      0.0        
    1.200     0.304      0.8821     25.0     d      0.375      
    0.905     0.600      0.8093     25.0     d      0.375      
    0.600     0.906      0.7456     25.0     d      0.375      
    0.380     1.140      0.6989     25.0     d      0.375      
    0.0       1.550      0.6283     25.0     d      0.0        
    2.100     0.0        0.9926     25.0     d      0.0        
    1.770     0.318      0.9277     25.0     d      0.375      
    1.440     0.641      0.8680     25.0     d      0.375      
    1.024     1.071      0.7924     25.0     d      0.375      
    0.727     1.411      0.7331     25.0     d      0.375      
    0.580     1.559      0.7142     25.0     d      0.375      
    2.856     0.0        1.0393     25.0     d      0.0        
    2.538     0.312      0.9874     25.0     d      0.375      
    2.214     0.633      0.9383     25.0     d      0.375      
    1.920     0.931      0.8950     25.0     d      0.375      
    1.596     1.261      0.8511     25.0     d      0.375      
    1.293     1.591      0.8067     25.0     d      0.375      
    3.342     0.0        1.0716     25.0     d      0.0        
    3.082     0.248      1.0369     25.0     d      0.375      
    2.856     0.467      1.0040     25.0     d      0.375      
    2.605     0.718      0.9700     25.0     d      0.375      
    2.240     1.077      0.9260     25.0     d      0.375      
    2.109     1.205      0.9110     25.0     d      0.375      
    3.851     0.0        1.1071     25.0     d      0.0         
    3.558     0.278      1.0726     25.0     d      0.375      
    3.253     0.581      1.0337     25.0     d      0.375      
    2.962     0.862      1.0020     25.0     d      0.375      
    2.674     1.148      0.9698     25.0     d      0.375      
    2.381     1.439      0.9392     25.0     d      0.375      
    4.540     0.0        1.1572     25.0     d      0.0         
    4.271     0.249      1.1312     25.0     d      0.375      
    3.985     0.516      1.1039     25.0     d      0.375      
    3.700     0.784      1.0775     25.0     d      0.375      
    3.431     1.041      1.0523     25.0     d      0.375      
    3.169     1.288      1.0299     25.0     d      0.375      

Notes and References

• Prefix m denotes molality; t - experimental temperature (^oC); osm - molal osmotic coefficient; ref. - source of data; weight - the weight given to the data point in the fit of the model (normalised).
• Sources: c - Y. C. Wu, R. M. Rush, and G. Scatchard (1968) J. Phys. Chem. 72, 4048-4053; d - V. K. Filippov and L. M. Cheremykh (1986) Vestn. Leningrad Univ. Ser. Fiz. Khim. 1, 47-50.

(4) Mean Activity Coefficients of NaCl (a)

   mNaCl     mNa2SO4     gamma       t    ref.   weight
    0.15      0.075      0.675     25.0    e      1.0          
    0.30      0.075      0.659     25.0    e      1.0          
    0.30      0.15       0.629     25.0    e      1.0          
    0.60      0.20       0.612     25.0    e      1.0          
    0.60      0.30       0.591     25.0    e      1.0          
    1.20      0.40       0.601     25.0    e      1.0          
    1.20      0.60       0.589     25.0    e      1.0          
    2.40      0.60       0.661     25.0    e      1.0          
    3.00      0.60       0.705     25.0    e      1.0          

Notes and References

• Prefix m denotes molality; gamma - mean molal activity coefficient of NaCl; t - experimental temperature (^oC); ref. - source of data; weight - the weight given to the data point in the fit of the model (normalised).
• Sources: e - P. Y. Tishchenko, A. S. Bychkov, A. Hrabeczy-Pall, K. Toth and E. Pungor (1992) J. Solut. Chem. 21, 261-274. (Cell 'A' only.)

(5) Mean Activity Coefficients of NaCl (b)

    mNaCl     mNa2SO4      Y             t     ref.   weight
    0.50000   0.00000   -0.1667     25.0     f      1.0        
    0.44700   0.01767   -0.1696     25.0     f      1.0        
    0.40415   0.03195   -0.1721     25.0     f      1.0        
    0.36880   0.04373   -0.1741     25.0     f      1.0        
    0.33910   0.05363   -0.1759     25.0     f      1.0        
    0.31390   0.06203   -0.1775     25.0     f      1.0        
    0.29215   0.06928   -0.1788     25.0     f      1.0         
    0.27320   0.07560   -0.1809     25.0     f      1.0  
    0.25655   0.08115   -0.1811     25.0     f      1.0  
    0.24185   0.08605   -0.1821     25.0     f      1.0  
    0.22875   0.09042   -0.1830     25.0     f      1.0  
    0.09100   0.13633   -0.1954     25.0     f      1.0  
    0.09260   0.13580   -0.1924     25.0     f      1.0  
    0.12710   0.12430   -0.1899     25.0     f      1.0  
    0.15625   0.11458   -0.1879     25.0     f      1.0  
    0.18115   0.10628   -0.1862     25.0     f      1.0  
    0.20270   0.09910   -0.1847     25.0     f      1.0  
    0.22150   0.09283   -0.1834     25.0     f      1.0  
    0.23810   0.08730   -0.1823     25.0     f      1.0  
    0.25280   0.08240   -0.1814     25.0     f      1.0  
    1.00000   0.00000   -0.1823     25.0     f      1.0  
    0.89320   0.03560   -0.1876     25.0     f      1.0  
    0.80700   0.06433   -0.1921     25.0     f      1.0  
    0.73600   0.08800   -0.1958     25.0     f      1.0  
    0.67650   0.10783   -0.1990     25.0     f      1.0  
    0.62580   0.12473   -0.2018     25.0     f      1.0  
    0.58230   0.13923   -0.2042     25.0     f      1.0  
    0.54440   0.15187   -0.2064     25.0     f      1.0  
    0.51110   0.16297   -0.2082     25.0     f      1.0  
    0.48170   0.17277   -0.2099     25.0     f      1.0  
    0.45540   0.18153   -0.2114     25.0     f      1.0  
    0.10320   0.29893   -0.2328     25.0     f      1.0  
    0.18620   0.27127   -0.2276     25.0     f      1.0  
    0.25650   0.24783   -0.2233     25.0     f      1.0  
    0.31510   0.22830   -0.2197     25.0     f      1.0  
    0.36510   0.21163   -0.2167     25.0     f      1.0  
    0.40830   0.19723   -0.2142     25.0     f      1.0  
    0.44600   0.18467   -0.2120     25.0     f      1.0  
    0.47910   0.17363   -0.2101     25.0     f      1.0  
    0.50860   0.16380   -0.2084     25.0     f      1.0  
    2.00000   0.00000   -0.1749     25.0     f      1.0  
    1.80100   0.06633   -0.1842     25.0     f      1.0  
    1.63820   0.12060   -0.1920     25.0     f      1.0  
    1.50220   0.16593   -0.1986     25.0     f      1.0  
    1.38720   0.20427   -0.2043     25.0     f      1.0  
    1.28840   0.23720   -0.2092     25.0     f      1.0  
    1.20280   0.26573   -0.2135     25.0     f      1.0  
    1.12800   0.29067   -0.2173     25.0     f      1.0  
    1.06180   0.31273   -0.2207     25.0     f      1.0  
    1.00280   0.33240   -0.2237     25.0     f      1.0  
    0.95040   0.34987   -0.2265     25.0     f      1.0  
    0.21240   0.59587   -0.2665     25.0     f      1.0  
    0.38400   0.53867   -0.2569     25.0     f      1.0  
    0.52540   0.49153   -0.2491     25.0     f      1.0  
    0.64420   0.45193   -0.2427     25.0     f      1.0  
    0.74520   0.41827   -0.2373     25.0     f      1.0  
    0.83240   0.38920   -0.2327     25.0     f      1.0  
    0.90800   0.36400   -0.2287     25.0     f      1.0  
    0.97460   0.34180   -0.2252     25.0     f      1.0  
    1.03340   0.32220   -0.2222     25.0     f      1.0  
    3.00000   0.00000   -0.1465     25.0     f      1.0  
    2.65680   0.11440   -0.1621     25.0     f      1.0  
    2.38410   0.20530   -0.1748     25.0     f      1.0  
    2.16210   0.27930   -0.1853     25.0     f      1.0  
    1.97790   0.34070   -0.1941     25.0     f      1.0  
    1.82280   0.39240   -0.2017     25.0     f      1.0  
    1.69020   0.43660   -0.2082     25.0     f      1.0  
    1.57530   0.47490   -0.2138     25.0     f      1.0  
    1.47540   0.50820   -0.2188     25.0     f      1.0  
    1.38720   0.53760   -0.2232     25.0     f      1.0  
    1.30890   0.56370   -0.2271     25.0     f      1.0  
    0.32010   0.89330   -0.2785     25.0     f      1.0  
    0.57840   0.80720   -0.2647     25.0     f      1.0  
    0.79140   0.73620   -0.2536     25.0     f      1.0  
    0.96990   0.67670   -0.2444     25.0     f      1.0  
    1.12170   0.62610   -0.2366     25.0     f      1.0  
    1.25250   0.58250   -0.2300     25.0     f      1.0  
    1.36620   0.54460   -0.2242     25.0     f      1.0  
    1.46610   0.51130   -0.2192     25.0     f      1.0  
    1.55430   0.48190   -0.2149     25.0     f      1.0  
    0.50000   0.00000   -0.1671     35.0     f       -   
    0.44755   0.01748   -0.1700     35.0     f       -   
    0.40510   0.03163   -0.1724     35.0     f       -   
    0.36995   0.04335   -0.1744     35.0     f       -   
    0.34045   0.05318   -0.1762     35.0     f       -   
    0.31530   0.06157   -0.1777     35.0     f       -   
    0.29360   0.06880   -0.1791     35.0     f       -    
    0.27470   0.07510   -0.1803     35.0     f       -   
    0.25810   0.08063   -0.1813     35.0     f       -   
    0.24335   0.08555   -0.1823     35.0     f       -   
    0.23025   0.08992   -0.1831     35.0     f       -   
    0.04830   0.15057   -0.1958     35.0     f       -   
    0.08810   0.13730   -0.1929     35.0     f       -   
    0.12145   0.12618   -0.1906     35.0     f       -   
    0.14980   0.11673   -0.1886     35.0     f       -   
    0.17420   0.10860   -0.1869     35.0     f       -   
    0.19540   0.10153   -0.1855     35.0     f       -   
    0.21405   0.09532   -0.1842     35.0     f       -   
    0.23050   0.08983   -0.1831     35.0     f       -   
    0.24520   0.08493   -0.1822     35.0     f       -   
    0.50000   0.00000   -0.1687     45.0     f       -   
    0.44790   0.01737   -0.1715     45.0     f       -   
    0.40560   0.03147   -0.1738     45.0     f       -   
    0.37060   0.04313   -0.1758     45.0     f       -   
    0.34120   0.05293   -0.1775     45.0     f       -   
    0.31610   0.06130   -0.1790     45.0     f       -   
    0.27555   0.07482   -0.1815     45.0     f       -   
    0.25895   0.08035   -0.1826     45.0     f       -   
    0.24420   0.08527   -0.1835     45.0     f       -   
    0.23100   0.08967   -0.1843     45.0     f       -   
    0.04925   0.15025   -0.1968     45.0     f       -   
    0.08965   0.13678   -0.1939     45.0     f       -   
    0.12340   0.12553   -0.1915     45.0     f       -   
    0.15205   0.11598   -0.1896     45.0     f       -   
    0.17665   0.10778   -0.1879     45.0     f       -   
    0.19795   0.10068   -0.1865     45.0     f       -   
    0.21665   0.09445   -0.1853     45.0     f       -   
    0.23320   0.08893   -0.1842     45.0     f       -   
    0.24790   0.08403   -0.1833     45.0     f       -   
    1.00000   0.00000   -0.1811     35.0     f       -   
    0.89340   0.03553   -0.1864     35.0     f       -   
    0.80730   0.06423   -0.1908     35.0     f       -   
    0.73630   0.08790   -0.1946     35.0     f       -   
    0.67680   0.10773   -0.1978     35.0     f       -   
    0.62620   0.12460   -0.2005     35.0     f       -   
    0.58270   0.13910   -0.2029     35.0     f       -   
    0.54480   0.15173   -0.2050     35.0     f       -   
    0.51150   0.16283   -0.2069     35.0     f       -   
    0.48210   0.17263   -0.2086     35.0     f       -   
    0.45590   0.18137   -0.2101     35.0     f       -   
    0.10430   0.29857   -0.2317     35.0     f       -   
    0.18890   0.27037   -0.2260     35.0     f       -   
    0.25890   0.24703   -0.2217     35.0     f       -   
    0.31770   0.22743   -0.2132     35.0     f       -   
    0.36800   0.21067   -0.2152     35.0     f       -   
    0.41430   0.19523   -0.2127     35.0     f       -   
    0.44900   0.18367   -0.2105     35.0     f       -   
    0.44230   0.18590   -0.2086     35.0     f       -   
    0.51170   0.16277   -0.2069     35.0     f       -   
    1.00000   0.00000   -0.1816     45.0     f       -   
    0.89390   0.03537   -0.1868     45.0     f       -   
    0.80820   0.06393   -0.1911     45.0     f       -   
    0.73740   0.08753   -0.1948     45.0     f       -   
    0.67810   0.10730   -0.1979     45.0     f       -   
    0.62760   0.12413   -0.2006     45.0     f       -   
    0.54620   0.15127   -0.2050     45.0     f       -   
    0.51300   0.16233   -0.2069     45.0     f       -   
    0.48350   0.17217   -0.2085     45.0     f       -   
    0.44730   0.18423   -0.2100     45.0     f       -   
    0.10310   0.29897   -0.2310     45.0     f       -   
    0.18700   0.27100   -0.2258     45.0     f       -   
    0.25650   0.24783   -0.2216     45.0     f       -   
    0.31510   0.22830   -0.2182     45.0     f       -   
    0.36510   0.21163   -0.2153     45.0     f       -   
    0.40830   0.19723   -0.2128     45.0     f       -   
    0.44600   0.18467   -0.2106     45.0     f       -   
    0.47910   0.17363   -0.2088     45.0     f       -   
    0.50810   0.16397   -0.2071     45.0     f       -   
    2.00000   0.00000   -0.1710     35.0     f       -   
    1.77800   0.07400   -0.1814     35.0     f       -   
    1.60060   0.13313   -0.1899     35.0     f       -   
    1.45520   0.18160   -0.1969     35.0     f       -   
    1.33400   0.22200   -0.2029     35.0     f       -   
    1.23160   0.25613   -0.2080     35.0     f       -   
    1.14360   0.28547   -0.2125     35.0     f       -   
    1.06740   0.31087   -0.2164     35.0     f       -   
    1.00080   0.33307   -0.2198     35.0     f       -   
    0.94200   0.35267   -0.2228     35.0     f       -   
    0.88960   0.37013   -0.2256     35.0     f       -   
    0.20700   0.59767   -0.2625     35.0     f       -   
    0.37500   0.54167   -0.2531     35.0     f       -   
    0.51440   0.49520   -0.2455     35.0     f       -   
    0.63160   0.45613   -0.2392     35.0     f       -   
    0.73180   0.42273   -0.2339     35.0     f       -   
    0.81820   0.39393   -0.2293     35.0     f       -   
    0.89360   0.36880   -0.2254     35.0     f       -   
    0.96000   0.34667   -0.2219     35.0     f       -   
    1.01900   0.32700   -0.2189     35.0     f       -   
    2.00000   0.00000   -0.1699     45.0     f       -   
    1.78260   0.07247   -0.1799     45.0     f       -   
    1.60800   0.13067   -0.1881     45.0     f       -   
    1.46440   0.17853   -0.1950     45.0     f       -   
    1.34440   0.21853   -0.2008     45.0     f       -   
    1.24260   0.25247   -0.2058     45.0     f       -   
    1.07920   0.30693   -0.2140     45.0     f       -   
    1.01260   0.32913   -0.2173     45.0     f       -   
    0.95360   0.34880   -0.2203     45.0     f       -   
    0.90120   0.36627   -0.2230     45.0     f       -   
    0.20860   0.59713   -0.2596     45.0     f       -   
    0.37780   0.54073   -0.2505     45.0     f       -   
    0.51780   0.49407   -0.2430     45.0     f       -   
    0.63540   0.45487   -0.2368     45.0     f       -   
    0.73580   0.42140   -0.2315     45.0     f       -   
    0.82260   0.39247   -0.2270     45.0     f       -   
    0.89800   0.36733   -0.2232     45.0     f       -   
    0.96440   0.34520   -0.2198     45.0     f       -   
    1.02340   0.32553   -0.2168     45.0     f       -   
    3.00000   0.00000   -0.1409     35.0     f       -   
    2.66280   0.11240   -0.1562     35.0     f       -   
    2.39370   0.20210   -0.1687     35.0     f       -   
    2.17410   0.27530   -0.1790     35.0     f       -   
    1.99140   0.33620   -0.1877     35.0     f       -   
    1.83690   0.38770   -0.1951     35.0     f       -   
    1.70460   0.43180   -0.2016     35.0     f       -   
    1.59030   0.46990   -0.2072     35.0     f       -   
    1.49010   0.50330   -0.2121     35.0     f       -   
    1.40190   0.53270   -0.2165     35.0     f       -   
    1.32360   0.55880   -0.2204     35.0     f       -   
    0.32670   0.89110   -0.2716     35.0     f       -   
    0.58920   0.80360   -0.2578     35.0     f       -   
    0.80610   0.73130   -0.2467     35.0     f       -   
    0.98490   0.67170   -0.2374     35.0     f       -   
    1.13790   0.62070   -0.2297     35.0     f       -   
    1.26690   0.57770   -0.2231     35.0     f       -   
    1.38300   0.53900   -0.2174     35.0     f       -   
    1.48290   0.50570   -0.2124     35.0     f       -   
    1.57110   0.47630   -0.2081     35.0     f       -   
    3.00000   0.00000   -0.1389     45.0     f       -   
    2.66700   0.11100   -0.1538     45.0     f       -   
    2.40060   0.19980   -0.1660     45.0     f       -   
    2.18250   0.27250   -0.1760     45.0     f       -   
    2.00070   0.33310   -0.1846     45.0     f       -   
    1.84710   0.38430   -0.1918     45.0     f       -   
    1.60080   0.46640   -0.2036     45.0     f       -   
    1.50090   0.49970   -0.2084     45.0     f       -   
    1.41270   0.52910   -0.2127     45.0     f       -   
    1.33440   0.55520   -0.2126     45.0     f       -   
    0.32010   0.89330   -0.2676     45.0     f       -   
    0.57840   0.80720   -0.2542     45.0     f       -   
    0.79110   0.73630   -0.2435     45.0     f       -   
    0.96960   0.67680   -0.2346     45.0     f       -   
    1.12140   0.62620   -0.2270     45.0     f       -   
    1.25220   0.58260   -0.2206     45.0     f       -   
    1.36590   0.54470   -0.2150     45.0     f       -   
    1.46550   0.51150   -0.2102     45.0     f       -   
    1.55400   0.48200   -0.2059     45.0     f       -   

Notes and References

• Prefix m denotes molality; Y - the logarithm (base 10) of the mean molal activity coefficient of NaCl; t - experimental temperature (^oC); ref. - source of data; weight - the weight given to the data point in the fit of the model (normalised).
• Sources: f - S. Sarada and J. Ananthaswamy (1990) J. Chem. Soc., Faraday Trans. 86, 81-84. (The measurements were made using ion-specific electrodes.)

(6) Osmotic Coefficients from Electrodynamic Balance Measurements

    mNaCl     mNa2SO4     osm        t      ref.     np   weight  
    2.8597    2.8597     1.0603     25.0     g(i)     1      -    
    1.9727    1.9727     0.8488     25.0     g(i)     1      -    
    2.2707    2.2707     0.9762     25.0     g(i)     1      -    
    3.2944    3.2944     1.1684     25.0     g(i)     1      -    
    3.9675    3.9675     1.2357     25.0     g(i)     1      -    
    4.7359    4.7359     1.2729     25.0     g(i)     1      -    
    2.0430    2.0430     0.8831     25.0     g(i)     2      -    
    2.1964    2.1964     0.9418     25.0     g(i)     2      -    
    2.4694    2.4694     1.0032     25.0     g(i)     2      -    
    3.0592    3.0592     1.1025     25.0     g(i)     2      -    
    3.5955    3.5955     1.1863     25.0     g(i)     2      -    
    4.1879    4.1879     1.2715     25.0     g(i)     2      -    
    5.1055    5.1055     1.2921     25.0     g(i)     2      -    
    3.3370    1.1123     0.9338     25.0     g(i)     1      -    
    2.8892    0.9631     0.9214     25.0     g(i)     1      -    
    3.6869    1.2290     1.0575     25.0     g(i)     1      -    
    4.3629    1.4543     1.1639     25.0     g(i)     1      -    
    4.9372    1.6457     1.2783     25.0     g(i)     1      -    
    5.7155    1.9052     1.3451     25.0     g(i)     1      -    
    6.4535    2.1512     1.4266     25.0     g(i)     1      -    
    3.2998    1.0999     1.1540     25.0     g(i)     2      -    
    2.9632    0.9877     0.9418     25.0     g(i)     2      -    
    4.0226    1.3408     1.1429     25.0     g(i)     2      -    
    4.8197    1.6066     1.2134     25.0     g(i)     2      -    
    5.6455    1.8818     1.2592     25.0     g(i)     2      -    
    0.8178    2.4533     0.7052     25.0     g(i)     1      -    
    1.0483    3.1448     0.8393     25.0     g(i)     1      -    
    1.2661    3.7983     0.9395     25.0     g(i)     1      -    
    1.5365    4.6095     1.0562     25.0     g(i)     1      -    
    1.8702    5.6105     1.1376     25.0     g(i)     1      -    
    2.2469    6.7407     1.1472     25.0     g(i)     1      -    
    1.1753    3.5258     0.8784     25.0     g(i)     2      -    
    0.9485    2.8456     0.8024     25.0     g(i)     2      -    
    1.3271    3.9812     0.9692     25.0     g(i)     2      -    
    1.5604    4.6811     1.0400     25.0     g(i)     2      -    
    1.8356    5.5067     1.0928     25.0     g(i)     2      -    
    2.0397    6.1190     1.1549     25.0     g(i)     2      -    
    2.2857    6.8572     1.2102     25.0     g(i)     2      -    
    2.2783    2.2783     0.9162     25.0     g(ii)    1      -    
    2.3343    2.3343     0.9634     25.0     g(ii)    1      -    
    2.5127    2.5127     1.0106     25.0     g(ii)    1      -    
    2.7519    2.7519     1.0524     25.0     g(ii)    1      -    
    3.0486    3.0486     1.1072     25.0     g(ii)    1      -    
    3.4752    3.4752     1.1400     25.0     g(ii)    1      -    
    3.9031    3.9031     1.1533     25.0     g(ii)    1      -    
    4.3718    4.3718     1.1173     25.0     g(ii)    1      -    
    4.8526    4.8526     1.0829     25.0     g(ii)    1      -    
    5.2305    5.2305     1.0627     25.0     g(ii)    1      -    
    5.6060    5.6060     1.0515     25.0     g(ii)    1      -    
    2.2624    2.2624     0.9493     25.0     g(ii)    2      -    
    2.3865    2.3865     0.9843     25.0     g(ii)    2      -    
    2.6061    2.6061     1.0131     25.0     g(ii)    2      -    
    2.8969    2.8969     1.0766     25.0     g(ii)    2      -    
    3.3335    3.3335     1.1279     25.0     g(ii)    2      -    
    3.7585    3.7585     1.1830     25.0     g(ii)    2      -    
    4.4022    4.4022     1.1208     25.0     g(ii)    2      -    
    4.9014    4.9014     1.0764     25.0     g(ii)    2      -    
    5.4395    5.4395     1.0462     25.0     g(ii)    2      -    
    5.9780    5.9780     1.0139     25.0     g(ii)    2      -    
    3.5053    1.1684     0.9836     25.0     g(ii)    1      -       
    3.5609    1.1870     1.0129     25.0     g(ii)    1      -    
    3.7181    1.2394     1.0412     25.0     g(ii)    1      -     
    4.1504    1.3835     1.1425     25.0     g(ii)    1      -     
    4.6593    1.5531     1.2167     25.0     g(ii)    1      -    
    5.1035    1.7012     1.2752     25.0     g(ii)    1      -    
    5.8053    1.9351     1.2982     25.0     g(ii)    1      -    
    6.4543    2.1514     1.2807     25.0     g(ii)    1      -    
    7.2122    2.4041     1.2399     25.0     g(ii)    1      -    
    7.7122    2.5708     1.2329     25.0     g(ii)    1      -    
    8.2732    2.7577     1.2158     25.0     g(ii)    1      -    
    8.6258    2.8753     1.2173     25.0     g(ii)    1      -    
    8.9580    2.9860     1.2264     25.0     g(ii)    1      -    
    3.3878    1.1293     0.9914     25.0     g(ii)    2      -    
    3.6173    1.2058     1.0236     25.0     g(ii)    2      -    
    4.1930    1.3977     1.1207     25.0     g(ii)    2      -    
    5.1824    1.7275     1.2338     25.0     g(ii)    2      -    
    5.9447    1.9816     1.2757     25.0     g(ii)    2      -    
    6.5430    2.1810     1.2638     25.0     g(ii)    2      -    
    6.9701    2.3234     1.2575     25.0     g(ii)    2      -    
    7.3957    2.4652     1.2515     25.0     g(ii)    2      -    
    7.6710    2.5570     1.2739     25.0     g(ii)    2      -    
    8.0033    2.6678     1.2744     25.0     g(ii)    2      -    
    8.3010    2.7670     1.2746     25.0     g(ii)    2      -    
    8.5815    2.8605     1.2813     25.0     g(ii)    2      -    

Notes and References

• Prefix m denotes molality; osm - molal osmotic coefficient; t - experimental temperature (^oC); ref. - source of data; weight - the weight given to the data point in the fit of the model (normalised).
• The measurements were made at room temperature (between 20 ^oC and 25.0 ^oC), and assumed to be at 25 ^oC.
• These data, which were used in the model described by Clegg et al. (1997), were not included in the fit of the AIM model, but are listed here for completeness.
• Sources: g(i) and g(ii) - C. K. Chan, Z. Liang, J. A. Zheng, S. L. Clegg and P. Brimblecombe (1997) Aerosol Science and Technology 27, 324- 344.